To delete the current user account, use the TLLoginComponent>>#deleteLoggedInUser method. Here's an example:
loginComponent deleteLoggedInUser.
To delete a specific user you can evaluate something like this:
(TLAuthenticationManager name: 'your-app-name')
deleteUserByUsername: 'the-username-to-delete'
where your-app-name is your application name as provided in TLLoginComponent>>#initialize.